Search results for "Propargyl bromide"

showing 2 items of 2 documents

Combining oxyanionic polymerization and click-chemistry: a general strategy for the synthesis of polyether polyol macromonomers

2014

We describe a synthetic pathway to tailor-made amphiphilic macromonomers by a combination of anionic ring-opening polymerization and copper-catalyzed azide–alkyne cycloaddition (CuAAC). Linear polyglycerol and poly(glyceryl glycerol) were synthesized in a controlled manner by anionic ring-opening polymerization of ethoxyethyl glycidyl ether or isopropylidene glyceryl glycidyl ether, respectively, with narrow and monomodal molecular weight distributions (Mw/Mn < 1.20) and molecular weights ranging from 850 g mol−1 to 2500 g mol−1. After end-capping with propargyl bromide and removal of the protecting groups, the hydrophilic precursors were quantitatively clicked to a series of hydrophobic az…

chemistry.chemical_classificationPolymers and PlasticsOrganic ChemistryRadical polymerizationBioengineeringBiochemistryCycloadditionchemistry.chemical_compoundchemistryPolymerizationPolymer chemistryAmphiphileClick chemistryCopolymerOrganic chemistryPropargyl bromideAlkylPolym. Chem.
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Evaluation of Antiradical Activity and Reducing Capacity of Synthesised Bispyridinium Dibromides Obtained by Quaternisation of 4-Pyridyl-1,4-dihydrop…

2015

New bispyridinium dibromides based on the 1,4-dihydropyridine (1,4-DHP) cycle were synthesised in the reaction between 4-pyridyl-1,4-DHP derivatives and propargyl bromide. It has been shown that variation of the substituent position on the pyridine as well as small changes in the electronic nature of the 1,4-DHP cycle as a result of the substituent nature at the 3 and 5 positions do not affect the course of the reaction and in all cases the corresponding bispyridinium dibromides 4a–e were formed. The antiradical activity, using 1,1-diphenyl-2-picrylhydrazine as a free radical scavenger, and the reducing capacity using phosphomolybdenum complexes have been evaluated for the newly synthesise…

Green chemistrychemistry.chemical_compoundReaction mechanismchemistryBiocatalysisPyridineSubstituentSupramolecular chemistryOrganic chemistryGeneral ChemistryPropargyl bromideFree radical scavengerMedicinal chemistryAustralian Journal of Chemistry
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